| 1 | R.E.M. | Losing My Religion | Out of Time (1991) | |
| 2 | Nirvana | Smells Like Teen Spirit | Nevermind (1991) | |
| 3 | Jesus Jones | Right Here, Right Now | Doubt (1991) | |
| 4 | EMF | Unbelievable | Schubert Dip (1991) | |
| 5 | Siouxsie and the Banshees | Kiss Them for Me | Superstition (1991) | |
| 6 | Seal | Crazy | Seal (1991) | |
| 7 | Big Audio Dynamite II | Rush | The Globe (1991) | |
| 8 | R.E.M. | Shiny Happy People | Out of Time (1991) | |
| 9 | Morrissey | Sing Your Life | Kill Uncle (1991) | |
| 10 | U2 | Mysterious Ways | Achtung Baby (1991) | |
| 11 | Sting | All This Time | The Soul Cages (1991) | |
| 12 | School of Fish | 3 Strange Days | School of Fish (1991) | |
| 13 | The Psychedelic Furs | Until She Comes | World Outside (1991) | |
| 14 | Too Much Joy | Crush Story | Cereal Killers (1991) | |
| 15 | Simple Minds | See the Lights | Real Life (1991) | |
| 16 | Electronic | Get the Message | Electronic (1991) | |
| 17 | Red Hot Chili Peppers | Give It Away | Blood Sugar Sex Magik (1991) | |
| 18 | The La’s | There She Goes | The La’s (1990) | |
| 19 | Alison Moyet | It Won't Be Long | Hoodoo (1991) | |
| 20 | Blur | There's No Other Way | Leisure (1991) | |
| 21 | Orchestral Manoeuvres in the Dark | Pandora's Box | Sugar Tax (1991) | |
| 22 | Material Issue | Valerie Loves Me | International Pop Overthrow (1991) | |
| 23 | Erasure | Chorus | Chorus (1991) | |
| 24 | Northside | Take 5 | Chicken Rhythms (1991) | |
| 25 | Divinyls | I Touch Myself | Divinyls (1991) | |
| 26 | The Farm | All Together Now | Spartacus (1990) | |
| 27 | R.E.M. | Radio Song | Out of Time (1991) | |
| 28 | Robyn Hitchcock and The Egyptians | So You Think You're in Love | Perspex Island (1991) | |
| 29 | The Shamen | Move Any Mountain (Progen 91) (Beat Edit) | En-Tact (1991) | |
| 30 | The Wonder Stuff | Caught in My Shadow | Never Loved Elvis (1991) | |
| 31 | Morrissey | That's Entertainment | Non-album Single (1991) | |
| 32 | U2 | The Fly | Achtung Baby (1991) | |
| 33 | Ride | Vapour Trail | Nowhere (1990) | |
| 34 | Jesus Jones | Real, Real, Real | Doubt (1991) | |
| 35 | Crowded House | It's Only Natural | Woodface (1991) | |
| 36 | Dramarama | Haven't Got a Clue | Vinyl (1991) | |
| 37 | Big Audio Dynamite II | The Globe | The Globe (1991) | |
| 38 | Voice of the Beehive | Monsters and Angels | Honey Lingers (1991) | |
| 39 | Violent Femmes | American Music | Why Do Birds Sing? (1991) | |
| 40 | Electronic | Feel Every Beat | Electronic (1991) | |
| 41 | Chapterhouse | Pearl | Whirlpool (1991) | |
| 42 | The Cult | Wild Hearted Son | Ceremony (1991) | |
| 43 | Jellyfish | That Is Why | Bellybutton (1990) | |
| 44 | EMF | Lies | Schubert Dip (1991) | |
| 45 | R.E.M. | Texarkana | Out of Time (1991) | |
| 46 | Lush | De-Luxe | Gala (1990) | |
| 47 | Seal | Future Love Paradise | Seal (1991) | |
| 48 | Billy Bragg | Sexuality | Don’t Try This at Home (1991) | |
| 49 | The Candyskins | For What It's Worth | Space I’m In (1991) | |
| 50 | The Farm | Groovy Train | Spartacus (1990) | |
| 51 | Too Much Joy | Long Haired Guys From England | Cereal Killers (1991) | |
| 52 | Morrissey | My Love Life | Non-album Single (1991) | |
| 53 | Ned's Atomic Dustbin | Grey Cell Green | God Fodder (1991) | |
| 54 | Orchestral Manoeuvres in the Dark | Sailing on the Seven Seas | Sugar Tax (1991) | |
| 55 | Jesus Jones | International Bright Young Thing | Doubt (1991) | |
| 56 | R.E.M. | Near Wild Heaven | Out of Time (1991) | |
| 57 | Gary Clail & On-U Sound System | Human Nature (On the Mix) (12" Version) | Emotional Hooligan (1991) | |
| 58 | Siouxsie and the Banshees | Shadowtime | Superstition (1991) | |
| 59 | EMF | Children | Schubert Dip (1991) | |
| 60 | Nirvana | Come As You Are | Nevermind (1991) | |
| 61 | Orchestral Manoeuvres in the Dark | Call My Name | Sugar Tax (1991) | |
| 62 | Nine Inch Nails | Down In It | Pretty Hate Machine (1989) | |
| 63 | Blue Train | All I Need Is You | Non-album Single (1991) | |
| 64 | The Smashing Pumpkins | Rhinoceros | Gish (1991) | |
| 65 | Elvis Costello | The Other Side of Summer | Mighty Like a Rose (1991) | |
| 66 | Primus | Jerry Was a Race Car Driver | Sailing the Seas of Cheese (1991) | |
| 67 | Erasure | Love To Hate You | Chorus (1991) | |
| 68 | Electronic | Tighten Up | Electronic (1991) | |
| 69 | Ned's Atomic Dustbin | Happy | God Fodder (1991) | |
| 70 | U2 | One | Achtung Baby (1991) | |
| 71 | Sting | The Soul Cages | The Soul Cages (1991) | |
| 72 | School of Fish | Wrong | School of Fish (1991) | |
| 73 | Morrissey | Our Frank | Kill Uncle (1991) | |
| 74 | My Life with the Thrill Kill Kult | Sex On Wheelz | Sexplosion! (1991) | |
| 75 | UB40 | Groovin' | Labour of Love II (1989) | |
| 76 | The Wonder Stuff | The Size of a Cow | Never Loved Elvis (1991) | |
| 77 | Right Said Fred | I'm Too Sexy | Up (1991) | |
| 78 | Hoodoo Gurus | Miss Freelove '69 | Kinky (1991) | |
| 79 | The Ocean Blue | Ballerina Out of Control | Cerulean (1991) | |
| 80 | The Psychedelic Furs | Don't Be a Girl | World Outside (1991) | |
| 81 | This Picture | Naked Rain | A Violent Impression (1991) | |
| 82 | Mary's Danish | Julie's Blanket (Pigsheadsnakeface) | Circa (1991) | |
| 83 | The Mock Turtles | Can You Dig It? | Turtle Soup (1990) | |
| 84 | Siouxsie and the Banshees | Fear (of the Unknown) | Superstition (1991) | |
| 85 | Kirsty MacColl | Walking Down Madison | Electric Landlady (1991) | |
| 86 | Jesus Jones | Welcome Back Victoria | Doubt (1991) | |
| 87 | Fishbone | Sunless Saturday | The Reality of My Surroundings (1991) | |
| 88 | Lloyd Cole | She's a Girl and I'm a Man | Don’t Get Weird on Me Babe (1991) | |
| 89 | Daniel Ash | This Love | Coming Down (1991) | |
| 90 | INXS | Bitter Tears | X (1990) | |
| 91 | Enya | Caribbean Blue | Shepherd Moons (1991) | |
| 92 | EMF | I Believe | Schubert Dip (1991) | |
| 93 | The Golden Palominos | Alive and Living Now | Drunk with Passion (1991) | |
| 94 | Transvision Vamp | If Looks Could Kill | Little Magnets Versus the Bubble of Babble (1991) | |
| 95 | Depeche Mode | Death's Door | Non-album Single (1991) | |
| 96 | Anthrax | Bring The Noise | Attack of the Killer B’s (1991) | |
| 97 | Talking Heads | Sax and Violins | Non-album Single (1991) | |
| 98 | The Orb | Little Fluffy Clouds | The Orb’s Adventures Beyond the Ultraworld (1991) | |
| 99 | Primal Scream | Movin' On Up | Screamadelica (1991) | |
| 100 | Squeeze | Satisfied | Play (1991) | |
| 101 | Happy Mondays | Bob's Yer Uncle | Pills ‘n’ Thrills and Bellyaches (1990) | |
| 102 | Candyland | Fountain o' Youth | Suck It and See (1991) | |
| 103 | Red Hot Chili Peppers | Breaking the Girl | Blood Sugar Sex Magik (1991) | |
| 104 | Saint Etienne | Only Love Can Break Your Heart | Foxbase Alpha (1991) | |
| 105 | Divinyls | Make Out Alright | Divinyls (1991) | |
| 106 | Pearl Jam | Alive | Ten (1991) | |
